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The papers contain for both Mary and Bernard Berenson biographical material, diaries, correspondence, and writings, both published and unpublished. There is also an extensive file of "Berensoniana," writings about Berenson and Villa I Tatti, but excluding reviews of publications. The papers are organized into seven series: I. Biographical, II. Collections, Villa I Tatti, and Harvard, III. Diaries, IV. Correspondence, V. Research and Writings, VI. Berensoniana, and VII. Photographs.
Address books and contact lists of Paul J. Sachs, created while collecting and teaching at the Fogg Museum. These contacts were used for personal use, student referrals, and professional contacts for the museum.